Recent progress on V2O5 nanowire nonwovens preparation and application in advanced electrochemical energy storage devices
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摘要: 五氧化二钒纳米纤维作为重要的钒基功能材料,在电化学储能领域有着重要应用。通过分析一维五氧化二钒纳米纤维及其聚集态材料在先进电化学储能器件应用领域的研究进展,结合近期研究前沿比较了不同五氧化二钒纳米纤维布合成方法的优缺点,认为采用降低尺寸和增加比表面积的策略将使其在电化学储能方面有更好的性能。同时,展望了V2O5纳米纤维布在未来先进电化学储能领域的发展前景,提出了其主要的发展和研究方向。Abstract: As an important V-based functional material, vanadium pentoxide (V2O5) nanofiber has a significant application in the field of electrochemical energy storage. We herein gave an overview of the one-dimensional (1D) V2O5-based materials for the application of advanced electrochemical energy storage and conversion, especially regarding the advantages and disadvantages of different synthetic methods of V2O5 nanowire nonwovens combined with recent research frontiers. It was considered that reducing the size and increasing the specific surface area will endow V2O5 with better performance in this field. Meanwhile, the development prospect of V2O5 nanofiber cloth in the field of advanced electrochemical energy storage in the future as well as the main development and research direction was provided.
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图 2 高有序V2O5纳米纤维泡沫制备、结构及其优异阻尼性能
Figure 2. Formation, structure, and performances (relative Young’s modulus and damping capacities) of single V2O5 nanofibers based highly ordered all-ceramic scaffolds[24]
图 3 V2O5纳米纤维层状晶格结构、原位锂化表征及储锂机理
Figure 3. Structural and lithiation progression characterizations of the pristine V2O5 nanowire as well as the proposed lithiation mechanism[39]
图 4 V2O5纳米纤维及其自支撑柔性石墨烯复合膜结构及其全固态锂离子电池正极材料性能(80℃)
Figure 4. Structure of V2O5-nanowire, freestanding flexible rGO/V2O5 composite paper and the performance of the as-prepared all-solid-state lithium–vanadium (rGO/V2O5/PEO-MIL-53(Al)-LiTFSI/Li) battery[6]
图 6 高有序V2O5纳米纤维泡沫衍生膜及其铝离子电池性能
Figure 6. Structures of the creased highly porous scaffold comprised of V2O5 nanowires and its aluminum-ion batteries (AIBs) performances[26]
图 7 V2O5纳米纤维/碳纳米管复合膜及其钠离子非对称超级电容器性能
Figure 7. Structures of the layered-V2O5-nanowires/CNTs nanocomposite film and the performance of the as-prepared Na-ion asymmetric supercapacitor[52]
图 8 V2O5纳米纤维膜及其银掺杂衍生物(SVO)的结构和电致变色性能
Figure 8. Structures of the V2O5 nanowire thin film and its Ag-doped derivative (SVO) as well as their electrochromic performance[10]
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